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Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning.
Содержание
Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning.
자료유형  
 학위논문
Control Number  
0017165150
International Standard Book Number  
9798346874058
Dewey Decimal Classification Number  
620.11
Main Entry-Personal Name  
Wei, Jingrui.
Publication, Distribution, etc. (Imprint  
[S.l.] : The University of Wisconsin - Madison., 2024
Publication, Distribution, etc. (Imprint  
Ann Arbor : ProQuest Dissertations & Theses, 2024
Physical Description  
94 p.
General Note  
Source: Dissertations Abstracts International, Volume: 86-06, Section: B.
General Note  
Advisor: Voyles, Paul M.
Dissertation Note  
Thesis (Ph.D.)--The University of Wisconsin - Madison, 2024.
Summary, Etc.  
요약Scanning transmission electron microscopy (STEM) has advanced the field of materials science by enabling atomic-scale structural and functional imaging. Beyond standard 2D imaging, higher dimensional data acquisition and analysis are enabling critical new sample insights. New challenges arise as well from the fast data streaming and big data volume. This thesis will discuss how advanced computational approaches and machine learning (ML) enhance the efficiency of STEM data interpretation with example topics. First, we demonstrate convolutional neural network (CNN) approaches for precise atom localization in high-resolution STEM images, establishing comprehensive benchmarks and investigating the relationship between model characteristics and performance across varying image qualities and content. Second, we introduce a deep learning-based electron counting method for ultrafast 4D-STEM detectors, utilizing a Faster-RCNN architecture to achieve accurate electron event detection at higher electron dose than previous methods. Third, a physics-informed regression model for STEM aberration measurement was developed to provide rapid aberration estimation for fine probe alignment or a starting point for sample phase reconstruction algorithms. Fourth, Z-contrast STEM imaging and 4D-STEM were used to investigate short-range order in high entropy carbides with different compositions and thermal treatment. The thesis concludes with a chapter speculating on future directions for research using ML in electron microscopy. Throughout this work, we highlight the importance of incorporating prior knowledge into the machine learning framework, ranging from data representation to model design, contributing to the broader field of quantitative electron microscopy and automation of STEM analysis.
Subject Added Entry-Topical Term  
Materials science.
Subject Added Entry-Topical Term  
Applied physics.
Subject Added Entry-Topical Term  
Computational physics.
Index Term-Uncontrolled  
Scanning transmission electron microscopy
Index Term-Uncontrolled  
Electron microscopy
Index Term-Uncontrolled  
Machine learning
Index Term-Uncontrolled  
Structure characterization
Index Term-Uncontrolled  
Electron dose
Added Entry-Corporate Name  
The University of Wisconsin - Madison Materials Science and Engineering
Host Item Entry  
Dissertations Abstracts International. 86-06B.
Electronic Location and Access  
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Control Number  
joongbu:657551
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