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Measuring Well-Width Dependent Disorder in Semiconductor Quantum Wells With Two-Dimensional Coherent Spectroscopy.
Measuring Well-Width Dependent Disorder in Semiconductor Quantum Wells With Two-Dimensional Coherent Spectroscopy.

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자료유형  
 학위논문
Control Number  
0017164379
International Standard Book Number  
9798384042396
Dewey Decimal Classification Number  
530
Main Entry-Personal Name  
Perez, Cesar.
Publication, Distribution, etc. (Imprint  
[S.l.] : University of Michigan., 2024
Publication, Distribution, etc. (Imprint  
Ann Arbor : ProQuest Dissertations & Theses, 2024
Physical Description  
108 p.
General Note  
Source: Dissertations Abstracts International, Volume: 86-03, Section: B.
General Note  
Advisor: Cundiff, Steven.
Dissertation Note  
Thesis (Ph.D.)--University of Michigan, 2024.
Summary, Etc.  
요약This thesis delves into the intricate realm of exciton physics within GaAs/Al0.3Ga0.7As quantum wells using Two-Dimensional Coherent Spectroscopy (2DCS), revealing novel insights into their coherent behaviors and interactions. Conducted in a box geometry with a pulsed laser operating at a repetition rate of 76 MHz and a pulse width of 100 fs within the near-infrared region, our investigation uncovers the distinctive characteristics of localized and delocalized excitons. It elucidates how factors such as disorder, quantum confinement, and external strain influence their coherent response and many-body interactions.Using two quantum well samples, one with a 10 nm well width and the other with a 20 nm well width featuring AlAs cladding layers to compensate for alloy concentration variations, we explore the impact of disorder and well-width variation on excitonic properties. We find that wider quantum wells promote delocalized excitons, affecting excitation-induced dephasing rates and thermal dephasing amplitudes, measured by keeping the sample temperature below 70 K. By applying the projection slice theorem, we directly measure time-dependent frequency correlations in the system, enhancing the accuracy of lineshape analysis in 2DCS experiments.Our study deviates from conventional approaches by directly measuring the frequency-frequency correlation function (FFCF), uncovering deviations from the Gauss-Markov approximation in wider quantum wells. We also investigate the effects of strain and quantum confinement on exciton dynamics, revealing strain-induced changes in dephasing rates and phonon activation energies. This thesis lays the groundwork for future research, suggesting avenues for studying biexciton dynamics in wide quantum wells, incorporating strain effects, and advancing theoretical models to better understand exciton-lattice interactions and improve lineshape analysis.
Subject Added Entry-Topical Term  
Physics.
Subject Added Entry-Topical Term  
Optics.
Subject Added Entry-Topical Term  
Atomic physics.
Subject Added Entry-Topical Term  
Analytical chemistry.
Index Term-Uncontrolled  
Quantum confinement
Index Term-Uncontrolled  
Spectroscopy
Index Term-Uncontrolled  
Quantum wells
Index Term-Uncontrolled  
Alloy concentration
Index Term-Uncontrolled  
Amplitudes
Added Entry-Corporate Name  
University of Michigan Applied Physics
Host Item Entry  
Dissertations Abstracts International. 86-03B.
Electronic Location and Access  
로그인을 한후 보실 수 있는 자료입니다.
Control Number  
joongbu:657239

MARC

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■035    ▼a(MiAaPQ)AAI31631182
■035    ▼a(MiAaPQ)umichrackham005613
■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a530
■1001  ▼aPerez,  Cesar.
■24510▼aMeasuring  Well-Width  Dependent  Disorder  in  Semiconductor  Quantum  Wells  With  Two-Dimensional  Coherent  Spectroscopy.
■260    ▼a[S.l.]▼bUniversity  of  Michigan.  ▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a108  p.
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-03,  Section:  B.
■500    ▼aAdvisor:  Cundiff,  Steven.
■5021  ▼aThesis  (Ph.D.)--University  of  Michigan,  2024.
■520    ▼aThis  thesis  delves  into  the  intricate  realm  of  exciton  physics  within  GaAs/Al0.3Ga0.7As  quantum  wells  using  Two-Dimensional  Coherent  Spectroscopy  (2DCS),  revealing  novel  insights  into  their  coherent  behaviors  and  interactions.  Conducted  in  a  box  geometry  with  a  pulsed  laser  operating  at  a  repetition  rate  of  76  MHz  and  a  pulse  width  of  100  fs  within  the  near-infrared  region,  our  investigation  uncovers  the  distinctive  characteristics  of  localized  and  delocalized  excitons.  It  elucidates  how  factors  such  as  disorder,  quantum  confinement,  and  external  strain  influence  their  coherent  response  and  many-body  interactions.Using  two  quantum  well  samples,  one  with  a  10  nm  well  width  and  the  other  with  a  20  nm  well  width  featuring  AlAs  cladding  layers  to  compensate  for  alloy  concentration  variations,  we  explore  the  impact  of  disorder  and  well-width  variation  on  excitonic  properties.  We  find  that  wider  quantum  wells  promote  delocalized  excitons,  affecting  excitation-induced  dephasing  rates  and  thermal  dephasing  amplitudes,  measured  by  keeping  the  sample  temperature  below  70  K.  By  applying  the  projection  slice  theorem,  we  directly  measure  time-dependent  frequency  correlations  in  the  system,  enhancing  the  accuracy  of  lineshape  analysis  in  2DCS  experiments.Our  study  deviates  from  conventional  approaches  by  directly  measuring  the  frequency-frequency  correlation  function  (FFCF),  uncovering  deviations  from  the  Gauss-Markov  approximation  in  wider  quantum  wells.  We  also  investigate  the  effects  of  strain  and  quantum  confinement  on  exciton  dynamics,  revealing  strain-induced  changes  in  dephasing  rates  and  phonon  activation  energies.  This  thesis  lays  the  groundwork  for  future  research,  suggesting  avenues  for  studying  biexciton  dynamics  in  wide  quantum  wells,  incorporating  strain  effects,  and  advancing  theoretical  models  to  better  understand  exciton-lattice  interactions  and  improve  lineshape  analysis.
■590    ▼aSchool  code:  0127.
■650  4▼aPhysics.
■650  4▼aOptics.
■650  4▼aAtomic  physics.
■650  4▼aAnalytical  chemistry.
■653    ▼aQuantum  confinement
■653    ▼aSpectroscopy
■653    ▼aQuantum  wells
■653    ▼aAlloy  concentration
■653    ▼aAmplitudes
■690    ▼a0748
■690    ▼a0752
■690    ▼a0605
■690    ▼a0486
■71020▼aUniversity  of  Michigan▼bApplied  Physics.
■7730  ▼tDissertations  Abstracts  International▼g86-03B.
■790    ▼a0127
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17164379▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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