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Measuring Well-Width Dependent Disorder in Semiconductor Quantum Wells With Two-Dimensional Coherent Spectroscopy.
Measuring Well-Width Dependent Disorder in Semiconductor Quantum Wells With Two-Dimensional Coherent Spectroscopy.
상세정보
- 자료유형
- 학위논문
- Control Number
- 0017164379
- International Standard Book Number
- 9798384042396
- Dewey Decimal Classification Number
- 530
- Main Entry-Personal Name
- Perez, Cesar.
- Publication, Distribution, etc. (Imprint
- [S.l.] : University of Michigan., 2024
- Publication, Distribution, etc. (Imprint
- Ann Arbor : ProQuest Dissertations & Theses, 2024
- Physical Description
- 108 p.
- General Note
- Source: Dissertations Abstracts International, Volume: 86-03, Section: B.
- General Note
- Advisor: Cundiff, Steven.
- Dissertation Note
- Thesis (Ph.D.)--University of Michigan, 2024.
- Summary, Etc.
- 요약This thesis delves into the intricate realm of exciton physics within GaAs/Al0.3Ga0.7As quantum wells using Two-Dimensional Coherent Spectroscopy (2DCS), revealing novel insights into their coherent behaviors and interactions. Conducted in a box geometry with a pulsed laser operating at a repetition rate of 76 MHz and a pulse width of 100 fs within the near-infrared region, our investigation uncovers the distinctive characteristics of localized and delocalized excitons. It elucidates how factors such as disorder, quantum confinement, and external strain influence their coherent response and many-body interactions.Using two quantum well samples, one with a 10 nm well width and the other with a 20 nm well width featuring AlAs cladding layers to compensate for alloy concentration variations, we explore the impact of disorder and well-width variation on excitonic properties. We find that wider quantum wells promote delocalized excitons, affecting excitation-induced dephasing rates and thermal dephasing amplitudes, measured by keeping the sample temperature below 70 K. By applying the projection slice theorem, we directly measure time-dependent frequency correlations in the system, enhancing the accuracy of lineshape analysis in 2DCS experiments.Our study deviates from conventional approaches by directly measuring the frequency-frequency correlation function (FFCF), uncovering deviations from the Gauss-Markov approximation in wider quantum wells. We also investigate the effects of strain and quantum confinement on exciton dynamics, revealing strain-induced changes in dephasing rates and phonon activation energies. This thesis lays the groundwork for future research, suggesting avenues for studying biexciton dynamics in wide quantum wells, incorporating strain effects, and advancing theoretical models to better understand exciton-lattice interactions and improve lineshape analysis.
- Subject Added Entry-Topical Term
- Physics.
- Subject Added Entry-Topical Term
- Optics.
- Subject Added Entry-Topical Term
- Atomic physics.
- Subject Added Entry-Topical Term
- Analytical chemistry.
- Index Term-Uncontrolled
- Quantum confinement
- Index Term-Uncontrolled
- Spectroscopy
- Index Term-Uncontrolled
- Quantum wells
- Index Term-Uncontrolled
- Alloy concentration
- Index Term-Uncontrolled
- Amplitudes
- Added Entry-Corporate Name
- University of Michigan Applied Physics
- Host Item Entry
- Dissertations Abstracts International. 86-03B.
- Electronic Location and Access
- 로그인을 한후 보실 수 있는 자료입니다.
- Control Number
- joongbu:657239
MARC
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■020 ▼a9798384042396
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■035 ▼a(MiAaPQ)umichrackham005613
■040 ▼aMiAaPQ▼cMiAaPQ
■0820 ▼a530
■1001 ▼aPerez, Cesar.
■24510▼aMeasuring Well-Width Dependent Disorder in Semiconductor Quantum Wells With Two-Dimensional Coherent Spectroscopy.
■260 ▼a[S.l.]▼bUniversity of Michigan. ▼c2024
■260 1▼aAnn Arbor▼bProQuest Dissertations & Theses▼c2024
■300 ▼a108 p.
■500 ▼aSource: Dissertations Abstracts International, Volume: 86-03, Section: B.
■500 ▼aAdvisor: Cundiff, Steven.
■5021 ▼aThesis (Ph.D.)--University of Michigan, 2024.
■520 ▼aThis thesis delves into the intricate realm of exciton physics within GaAs/Al0.3Ga0.7As quantum wells using Two-Dimensional Coherent Spectroscopy (2DCS), revealing novel insights into their coherent behaviors and interactions. Conducted in a box geometry with a pulsed laser operating at a repetition rate of 76 MHz and a pulse width of 100 fs within the near-infrared region, our investigation uncovers the distinctive characteristics of localized and delocalized excitons. It elucidates how factors such as disorder, quantum confinement, and external strain influence their coherent response and many-body interactions.Using two quantum well samples, one with a 10 nm well width and the other with a 20 nm well width featuring AlAs cladding layers to compensate for alloy concentration variations, we explore the impact of disorder and well-width variation on excitonic properties. We find that wider quantum wells promote delocalized excitons, affecting excitation-induced dephasing rates and thermal dephasing amplitudes, measured by keeping the sample temperature below 70 K. By applying the projection slice theorem, we directly measure time-dependent frequency correlations in the system, enhancing the accuracy of lineshape analysis in 2DCS experiments.Our study deviates from conventional approaches by directly measuring the frequency-frequency correlation function (FFCF), uncovering deviations from the Gauss-Markov approximation in wider quantum wells. We also investigate the effects of strain and quantum confinement on exciton dynamics, revealing strain-induced changes in dephasing rates and phonon activation energies. This thesis lays the groundwork for future research, suggesting avenues for studying biexciton dynamics in wide quantum wells, incorporating strain effects, and advancing theoretical models to better understand exciton-lattice interactions and improve lineshape analysis.
■590 ▼aSchool code: 0127.
■650 4▼aPhysics.
■650 4▼aOptics.
■650 4▼aAtomic physics.
■650 4▼aAnalytical chemistry.
■653 ▼aQuantum confinement
■653 ▼aSpectroscopy
■653 ▼aQuantum wells
■653 ▼aAlloy concentration
■653 ▼aAmplitudes
■690 ▼a0748
■690 ▼a0752
■690 ▼a0605
■690 ▼a0486
■71020▼aUniversity of Michigan▼bApplied Physics.
■7730 ▼tDissertations Abstracts International▼g86-03B.
■790 ▼a0127
■791 ▼aPh.D.
■792 ▼a2024
■793 ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17164379▼nKERIS▼z이 자료의 원문은 한국교육학술정보원에서 제공합니다.
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