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Scanning Tunneling Microscopy Characterization of Two-Dimensional Magnetic, Topological Heterostructures.
Содержание
Scanning Tunneling Microscopy Characterization of Two-Dimensional Magnetic, Topological Heterostructures.
자료유형  
 학위논문
Control Number  
0017164989
International Standard Book Number  
9798384460169
Dewey Decimal Classification Number  
530
Main Entry-Personal Name  
Goff, Bradley M.
Publication, Distribution, etc. (Imprint  
[S.l.] : The Ohio State University., 2024
Publication, Distribution, etc. (Imprint  
Ann Arbor : ProQuest Dissertations & Theses, 2024
Physical Description  
268 p.
General Note  
Source: Dissertations Abstracts International, Volume: 86-04, Section: B.
General Note  
Advisor: Gupta, Jay A.
Dissertation Note  
Thesis (Ph.D.)--The Ohio State University, 2024.
Summary, Etc.  
요약Introducing magnetism to topological insulators can produce a variety of interesting macroscopic quantum phenomena and open new paradigms for energy-efficient and high-performance computing. This dissertation presents the first scanning tunneling microscopy study of a novel heterostructure consisting of the two-dimensional itinerant ferromagnet Fe3GeTe2 (FGT) and the topological insulator Bi2Te3. The electronic and topographic structure is characterized with atomic resolution, providing insights into the interface between magnetism and topology.I show that FGT rotationally aligns to the Bi2Te3 and both materials are unstrained with an electronic density of states identical to their bulk counterparts. Bi2Te3 is confirmed to retain its topological properties via quasiparticle inference imaging of the topological surface state. FGT is shown to retain its ferromagnetic properties down to the monolayer limit via MCD measurements.In addition, this dissertation details significant development towards a nanoscale magnetism measurement technique, FMR-STM. I demonstrate a reliable and efficient procedure to measure the transfer function to a sample with a strongly nonlinear I(V) curve. The transfer function is used to apply radio frequency (RF) excitations from 1 to 20 GHz with constant amplitude at the tunnel junction. I show a measurement of the thermoelastic expansion due to heating from the RF absorption associated with cable resonances. This is an important background signal for future FMR measurements. Additionally, I report the discovery of novel RF effects on field emission resonance (FER) states and demonstrate a proof-of-principle measurement of the relative transfer function utilizing the shift in FER energies.Lastly, I present software that I developed: MacroQueue. It provides a simple GUI to allow users to automate STM measurements throughout the entire parameter space without requiring coding. Currently, MacroQueue includes functions to control the 3 most common commercial STM systems - CreaTec, RHK, and Scienta Omicron - and can be extended to automate any system controllable via Python. This software is currently in active use in several laboratories at The Ohio State University and the NSF NeXUS Facility.
Subject Added Entry-Topical Term  
Condensed matter physics.
Subject Added Entry-Topical Term  
Physics.
Subject Added Entry-Topical Term  
Quantum physics.
Index Term-Uncontrolled  
2D materials
Index Term-Uncontrolled  
Magnetic properties
Index Term-Uncontrolled  
Topological heterostructures
Index Term-Uncontrolled  
Topological insulators
Added Entry-Corporate Name  
The Ohio State University Physics
Host Item Entry  
Dissertations Abstracts International. 86-04B.
Electronic Location and Access  
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Control Number  
joongbu:655495
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